Advanced Materials, Vol.24, No.46, 6169-6174, 2012
Triplet Exciton Dissociation in Singlet Exciton Fission Photovoltaics
Triplet exciton dissociation in singlet exciton fission devices with three classes of acceptors are characterized: fullerenes, perylene diimides, and PbS and PbSe colloidal nanocrystals. Using photocurrent spectroscopy and a magnetic field probe it is found that colloidal PbSe nanocrystals are the most promising acceptors, capable of efficient triplet exciton dissociation and long wavelength absorption.