Enhanced electrochemical oxidation of dye wastewater with Fe2O3 supported catalyst

Lin Yue; Kaihong Wang; Jianbo Guo; Jingliang Yang; Xiao Luo; Jing Lian; Li Wang

Journal of Industrial and Engineering Chemistry, Vol.20, No.2, 725-731, March, 2014

DOI10.1016/j.jiec.2013.06.001 Export Citation

Enhanced electrochemical oxidation of dye wastewater with Fe2O3 supported catalyst

Lin Yue, Kaihong Wang, Jianbo Guo^†, Jingliang Yang, Xiao Luo, Jing Lian, and Li Wang

College of Environmental Science and Engineering, Hebei University of Science and Technology, Shi Jiazhuang 050018, China

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Electrochemical oxidation of Acid Red 3R was investigated in the presence of Fe2O3/g-Al2O3 as Fenton-like catalyst in the reactor. The results showed that the catalyst had catalytic activity in the electrochemical process. Under the optimal conditions, the decolorization efficiency reached 77.2% in 100 min. UV-vis spectrum and LC-MS analysis revealed that the dye molecule was firstly decomposed to aromatic intermediates, further degraded to ring opening products and finally mineralized. The azo dye degradation might be attributed to strong oxidant ㆍOH that produced from the synergetic effect of between Fe2O3/g-Al2O3 catalyst and electrochemical system.

Keywords:Electrochemical oxidation;Azo dye;Fe2O3;Supported catalyst

[References]

Sirianuntapiboon S, Sansak J, J. Hazard. Mater., 159(2-3), 404 (2008)
El-Gohary F, Tawfik A, Desalination, 249(3), 1159 (2009)
Sirianuntapiboon S, Srisornsak P, Bioresour. Technol., 98(5), 1057 (2007)
Wijetunga S, Li XF, Jian C, J. Hazard. Mater., 177(1-3), 792 (2010)
Arslan-Alaton I, J. Environ. Manage., 82, 145 (2007)
Yasar A, Ahmad N, Khan AAA, Yousaf A, J. Environ. Sci., 19, 1183 (2007)
Ghoneim MM, El-Desoky HS, Zidan NM, Desalination, 274(1-3), 22 (2011)
Ma HZ, Wang B, Luo XY, J. Hazard. Mater., 149(2), 492 (2007)
Georgiou D, Metallinou C, Aivasidis A, et al., Biochem. Eng. J., 19, 75 (2004)
Talarposhti AM, Donnelly T, Anderson GK, Water Res., 35, 425 (2001)
Khehra MS, Saini HS, Sharma DK, et al., Dyes Pigment., 70, 1 (2006)
Gottlieb A, Shaw C, Smith S, et al., J. Biotechnol., 101, 49 (2003)
Anouzla A, Abrouki Y, Souabi S, Safi M, Rhbal H, J. Hazard. Mater., 166(2-3), 1302 (2009)
Veliev EV, Ozturk T, Veli S, et al., Pol. J. Environ. Stu., 15, 347 (2006)
Devi LG, Kumar SG, Reddy KM, Munikrishnappa C, J. Hazard. Mater., 164(2-3), 459 (2009)
Patel R, Suresh S, J. Hazard. Mater., 137(3), 1729 (2006)
Zhang H, Duan L, Zhang Y, et al., Dyes, 65, 39 (2005)
Zhou MH, Lei LC, Chemosphere, 65, 1197 (2006)
Xiong Y, Karlsson HT, Adv. Environ. Res., 7, 139 (2002)
Ma HZ, Zhuo QF, Wang B, Chem. Eng. J., 155(1-2), 248 (2009)
Kariyajjanavar P, Jogttappa N, Nayaka YA, J. Hazard. Mater., 190(1-3), 952 (2011)
Yang CL, McGarrahan J, J. Hazard. Mater., 127(1-3), 40 (2005)
Parsa JB, Rezaei M, Soleymani AR, J. Haz, 168(2-3), 997 (2009)
Can OT, Bayramoglu M, Kobya M, Ind. Eng. Chem. Res., 42(14), 3391 (2003)
Lin SH, Peng CF, Water Res., 28, 277 (2003)
Khataee AR, Vatanpour V, Ghadim ARA, J. Hazard. Mater., 161(2-3), 1225 (2009)
Pirkanniemi K, Sillanpaa M, Chemosphere, 48, 1047 (2002)
Hsueh CL, Huang YH, Wang CC, et al., Chemosphere, 58, 1409 (2005)
Lodha B, Chaudhari S, J. Hazard. Mater., 148(1-2), 459 (2007)
Chai XS, Hou QX, Luo Q, Zhu JY, Anal. Chim. Acta, 507, 281 (2004)
Ramirez E GG, Theng BKG, Mora ML, Appl. Clay Sci., 47, 182 (2010)
Ji F, Li CL, Zhang JH, Deng L, Desalination, 269(1-3), 284 (2011)
Khataee AR, Pons MN, Zahraa O, J. Hazard. Mater., 168(1), 451 (2009)

[Referenced By]

[1] Sirianuntapiboon S, Sansak J, J. Hazard. Mater., 159(2-3), 404 (2008)

[2] El-Gohary F, Tawfik A, Desalination, 249(3), 1159 (2009)

[3] Sirianuntapiboon S, Srisornsak P, Bioresour. Technol., 98(5), 1057 (2007)

[4] Wijetunga S, Li XF, Jian C, J. Hazard. Mater., 177(1-3), 792 (2010)

[5] Arslan-Alaton I, J. Environ. Manage., 82, 145 (2007)

[6] Yasar A, Ahmad N, Khan AAA, Yousaf A, J. Environ. Sci., 19, 1183 (2007)

[7] Ghoneim MM, El-Desoky HS, Zidan NM, Desalination, 274(1-3), 22 (2011)

[8] Ma HZ, Wang B, Luo XY, J. Hazard. Mater., 149(2), 492 (2007)

[9] Georgiou D, Metallinou C, Aivasidis A, et al., Biochem. Eng. J., 19, 75 (2004)

[10] Talarposhti AM, Donnelly T, Anderson GK, Water Res., 35, 425 (2001)

[11] Khehra MS, Saini HS, Sharma DK, et al., Dyes Pigment., 70, 1 (2006)

[12] Gottlieb A, Shaw C, Smith S, et al., J. Biotechnol., 101, 49 (2003)

[13] Anouzla A, Abrouki Y, Souabi S, Safi M, Rhbal H, J. Hazard. Mater., 166(2-3), 1302 (2009)

[14] Veliev EV, Ozturk T, Veli S, et al., Pol. J. Environ. Stu., 15, 347 (2006)

[15] Devi LG, Kumar SG, Reddy KM, Munikrishnappa C, J. Hazard. Mater., 164(2-3), 459 (2009)

[16] Patel R, Suresh S, J. Hazard. Mater., 137(3), 1729 (2006)

[17] Zhang H, Duan L, Zhang Y, et al., Dyes, 65, 39 (2005)

[18] Zhou MH, Lei LC, Chemosphere, 65, 1197 (2006)

[19] Xiong Y, Karlsson HT, Adv. Environ. Res., 7, 139 (2002)

[20] Ma HZ, Zhuo QF, Wang B, Chem. Eng. J., 155(1-2), 248 (2009)

[21] Kariyajjanavar P, Jogttappa N, Nayaka YA, J. Hazard. Mater., 190(1-3), 952 (2011)

[22] Yang CL, McGarrahan J, J. Hazard. Mater., 127(1-3), 40 (2005)

[23] Parsa JB, Rezaei M, Soleymani AR, J. Haz, 168(2-3), 997 (2009)

[24] Can OT, Bayramoglu M, Kobya M, Ind. Eng. Chem. Res., 42(14), 3391 (2003)

[25] Lin SH, Peng CF, Water Res., 28, 277 (2003)

[26] Khataee AR, Vatanpour V, Ghadim ARA, J. Hazard. Mater., 161(2-3), 1225 (2009)

[27] Pirkanniemi K, Sillanpaa M, Chemosphere, 48, 1047 (2002)

[28] Hsueh CL, Huang YH, Wang CC, et al., Chemosphere, 58, 1409 (2005)

[29] Lodha B, Chaudhari S, J. Hazard. Mater., 148(1-2), 459 (2007)

[30] Chai XS, Hou QX, Luo Q, Zhu JY, Anal. Chim. Acta, 507, 281 (2004)

[31] Ramirez E GG, Theng BKG, Mora ML, Appl. Clay Sci., 47, 182 (2010)

[32] Ji F, Li CL, Zhang JH, Deng L, Desalination, 269(1-3), 284 (2011)

[33] Khataee AR, Pons MN, Zahraa O, J. Hazard. Mater., 168(1), 451 (2009)