Journal of Chemical Physics, Vol.104, No.3, 1159-1162, 1996
Temporally 2-Dimensional Femtosecond Spectroscopy of Binary Mixture of Cs2
We have studied the inhomogeneity of the low-frequency modes of binary mixtures of CS2 with various cosolvents by the temporally two-dimensional spectroscopy with femtosecond pulses. The inhomogeneity in the underdamped mode is found to be decreased upon dilution for all the solvents investigated.
Keywords:LIQUID CARBON-DISULFIDE;INTERACTION-INDUCED SPECTRA;STIMULATED LIGHT-SCATTERING;OPTICAL KERR DYNAMICS;MOLECULAR-DYNAMICS;PHOTON-ECHOES;LINE-SHAPES;ACETONITRILE;TEMPERATURE;SELECTIVITY