Journal of Chemical Physics, Vol.107, No.3, 927-931, 1997
Instability Scenarios for Doped He-4 Clusters
In the frame of finite range density functional (FRDF) theory, we review the systematics of energetic features of He-4(N) clusters doped with atomic or molecular impurities, as well as the instability scenario of their collective motions. It is shown that for drops up to N=500, the predictions of FRDF theory are coincident with those arising from microscopic many-body calculations that employ variational or diffusion Monte Carlo methods. For larger drops, the present description predicts a smooth approach to zero of the collective energies, a scenario that appears to support the most recent experimental data and microscopic calculations that demonstrate that the impurity is located within the bulk of the drop.