Journal of Crystal Growth, Vol.378, 442-445, 2013
Structural properties of ultra-low density nanoholes for the generation of well-separated GaAs quantum dots
We apply the local droplet etching (LDE) technique in a conventional molecular beam epitaxy system for self-organized nanohole formation on AlGaAs surfaces. By optimizing the arsenic flux during the Al droplet deposition the hole density can be reduced down to the 10(6) cm(-2) regime. The nanohole shape and density are tunable in a wide range by the amount of droplet material deposited and the initial holes are customized by overgrowth with AlGaAs of varied thickness. Nanoholes with controlled depths from 30 down to a few nanometers are fabricated, while the ultra-low density is sustained. These nanoholes are filled with GaAs to form well separated GaAs QDs, with size precisely controlled by the filling level. Studies of the optical emission of single dots exhibit sharp excitonic lines at low and a clear shell structure at high excitation power. In particular, the quantization energies in dependence of the QD size are measured. (c) 2012 Elsevier B.V. All rights reserved.
Keywords:Atomic force microscopy;Nanostructures;Molecular beam epitaxy;Semiconducting III-V materials