Simultaneous ultra-trace palladium(II) detection and recovery from wastewater using new class meso-adsorbent

Md. Rabiul Awual; Md. Abdul Khaleque; Yeasmin Ratna; Hussein Znad

Journal of Industrial and Engineering Chemistry, Vol.21, 405-413, January, 2015

DOI10.1016/j.jiec.2014.02.053 Export Citation

Simultaneous ultra-trace palladium(II) detection and recovery from wastewater using new class meso-adsorbent

Md. Rabiul Awual^†, Md. Abdul Khaleque¹, Yeasmin Ratna², and Hussein Znad³

Actinide Coordination Chemistry Group, Quantum Beam Science Directorate (QuBS), Japan Atomic Energy Agency (SPring-8), Hyogo 679-5148, Japan
¹Department of Environmental Science, School of Environmental Science and Management, Independent University, Bangladesh, Dhaka 1229, Bangladesh
²Department of Chemistry, University of Dhaka, Dhaka 1000, Bangladesh
³Department of Chemical Engineering, Curtin University, GPO BoxU1987, Perth, WA 6845, Australia

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A novel functionalized mesoporous silica based meso-adsorbent was prepared for simple, efficient and rapid determination, sorption and recovery of trace palladium(II) in wastewater. The meso-adsorbent was prepared by indirect immobilization of ((3-(3-(methoxycarbonyl)benzylidene)hydrazinyl)benzoic acid) onto the cage-pored mesoporous silica. The optimum conditions were measured as a function of solution acidity, contact time, ion selectivity and adsorption isotherms models. The data revealed that meso-adsorbent offered simple and one-step procedure without using high tech instruments. The determined detection limit and sorption capacity were 0.11 μg/L and 184.50 mg/g, respectively. The meso-adsorbent can be repeatedly recycled without deterioration of the unique mesostructures and maintaining the same functionality for detection/sorption operations in next uses.

Keywords:Meso-adsorbent;Palladium(II);Detection and recovery;Selectivity and sensitivity;Reuses

[References]

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Zhou LM, Liu JH, Liu ZR, J. Hazard. Mater., 172(1), 439 (2009)
Tunceli A, Turker AR, Anal. Sci., 16, 81 (2000)
Barakat MA, Mahmoud MHH, Mahrous YS, Appl. Catal. A: Gen., 301(2), 182 (2006)
Gaita R, Al-Bazi SJ, Talanta, 42, 249 (1995)
Kolarik Z, Renard EV, Platinum Met. Rev., 47, 123 (2003)
International Programme on Chemical Safety, Palladium; Environmental Health Criteria Series 226, World Health Organization, Geneva, 2002.
Merget R, Rosner G, Sci. Total Environ., 270, 165 (2001)
Leopold K, Maier M, Weber S, Schuster M, Environ. Pollut., 156, 341 (2008)
Whiteley JD, Water Air Soil Pollut., 160, 77 (2005)
Van Meel K, Smekens A, Behets M, Kazandjian P, Van Grieken R, Anal. Chem., 79, 6383 (2007)
Dimitrova B, Benkhedda K, Ivanova E, Adams F, J. Anal. Atom. Spectrom., 19, 1394 (2004)
Awual MR, Yaita T, Sens. Actuators B-Chem., 183, 332 (2013)
Awual MR, Yaita T, El-Safty SA, Shiwaku H, Okamoto Y, Suzuki S, Chem. Eng. J., 222, 172 (2013)
Awual MR, Rahman IMM, Yaita T, Khaleque MA, Ferdows M, Chem. Eng. J., 236, 100 (2014)
Hann S, Rudolph E, Kollensperger G, Reiter C, in: Zereini F, Alt F (Eds.), Analytical Methods, Environmental Assessment and Health Effects, Springer, Heidelberg, 2006, p. 73.
Hall GEM, Pelchat JC, J. Anal. Atom. Spectrom., 8, 1059 (1993)
Nguyen HT, Masayuki W, Takaumi K, Solvent Extr. Ion Exch., 25, 407 (2007)
Godlewska-Zylkiewicz B, Lesniewska B, Gasiewska U, Hulanicki A, Anal. Lett., 33, 2805 (2000)
Birinci E, Gulfen M, Aydın AO, Hydrometallurgy, 95, 15 (2009)
Sadyrbaeva TZ, J. Membr. Sci., 275(1-2), 195 (2006)
Maruyama T, Matsushita H, Shimada Y, Kamata I, Hanaki M, Sonokawa S, Kamiya N, Goto M, Environ. Technol., 41, 1359 (2007)

[Referenced By]

[1] Zhou LM, Xu JP, Liang XZ, Liu ZR, J. Hazard. Mater., 182(1-3), 518 (2010)

[2] Zhou LM, Liu JH, Liu ZR, J. Hazard. Mater., 172(1), 439 (2009)

[3] Tunceli A, Turker AR, Anal. Sci., 16, 81 (2000)

[4] Barakat MA, Mahmoud MHH, Mahrous YS, Appl. Catal. A: Gen., 301(2), 182 (2006)

[5] Gaita R, Al-Bazi SJ, Talanta, 42, 249 (1995)

[6] Kolarik Z, Renard EV, Platinum Met. Rev., 47, 123 (2003)

[7] International Programme on Chemical Safety, Palladium; Environmental Health Criteria Series 226, World Health Organization, Geneva, 2002.

[8] Merget R, Rosner G, Sci. Total Environ., 270, 165 (2001)

[9] Leopold K, Maier M, Weber S, Schuster M, Environ. Pollut., 156, 341 (2008)

[10] Whiteley JD, Water Air Soil Pollut., 160, 77 (2005)

[11] Van Meel K, Smekens A, Behets M, Kazandjian P, Van Grieken R, Anal. Chem., 79, 6383 (2007)

[12] Dimitrova B, Benkhedda K, Ivanova E, Adams F, J. Anal. Atom. Spectrom., 19, 1394 (2004)

[13] Awual MR, Yaita T, Sens. Actuators B-Chem., 183, 332 (2013)

[14] Awual MR, Yaita T, El-Safty SA, Shiwaku H, Okamoto Y, Suzuki S, Chem. Eng. J., 222, 172 (2013)

[15] Awual MR, Rahman IMM, Yaita T, Khaleque MA, Ferdows M, Chem. Eng. J., 236, 100 (2014)

[16] Hann S, Rudolph E, Kollensperger G, Reiter C, in: Zereini F, Alt F (Eds.), Analytical Methods, Environmental Assessment and Health Effects, Springer, Heidelberg, 2006, p. 73.

[17] Hall GEM, Pelchat JC, J. Anal. Atom. Spectrom., 8, 1059 (1993)

[18] Nguyen HT, Masayuki W, Takaumi K, Solvent Extr. Ion Exch., 25, 407 (2007)

[19] Godlewska-Zylkiewicz B, Lesniewska B, Gasiewska U, Hulanicki A, Anal. Lett., 33, 2805 (2000)

[20] Birinci E, Gulfen M, Aydın AO, Hydrometallurgy, 95, 15 (2009)

[21] Sadyrbaeva TZ, J. Membr. Sci., 275(1-2), 195 (2006)

[22] Maruyama T, Matsushita H, Shimada Y, Kamata I, Hanaki M, Sonokawa S, Kamiya N, Goto M, Environ. Technol., 41, 1359 (2007)