Hydrodynamics of collision interactions between a particle and gas-liquid interface such as droplet/film is of keen interest in many engineering applications. The collision interaction between a suspended liquid (water) film of thickness 3.41 +/- 0.04 mm and an impacting hydrophilic particle (glass ballotini) of different diameters (1.1-3.0 mm) in low particle impact Weber number (We = rho(l)nu(2)(p)d(p)/sigma) range (1.4-33) is reported. Two distinct outcomes were observed-particle retention in the film at lower Weber number and complete penetration of the film toward higher Weber number cases. A collision parameter was defined based on energy balance approach to demarcate these two interaction regimes which agreed reasonably well with the experimental outcomes. It was shown that the liquid ligament forming in the complete penetration cases breaks up purely by "dripping/end pinch-off" mechanism and not due to capillary wave instability. An analytical model based on energy balance approach was proposed to determine the liquid mass entrainment associated with the ligament which compared well with the experimental measurements. A good correlation between the % film mass entrained and the particle Bond number (Bo = rho(l)gd(p)(2)/sigma) was obtained which indicated a dependency of Bo(1.72). Computationally, a three-dimensional CFD model was developed to simulate these interactions using different contact angle boundary conditions which in general showed reasonable agreement with experiment but also indicated deficiency of a constant contact angle value to depict the interaction physics in entirety. The computed force profiles from computational fluid dynamics (CFD) model suggest dominance of the pressure force over the viscous force almost by an order of magnitude in all the Weber number cases studied. (C) 2015 American Institute of Chemical Engineers