Agricultural residues (wheat/barley/oat straw) can be used to produce charcoal, which can then be either landfilled off-site or spread on the agricultural field as a means for sequestering carbon. One centralized and five portable charcoal production technologies were explored in this paper. The centralized system produced 747.95 kg-CO(2)eq/tonne-straw and sequestered 0.204 t-C/t-straw. The portable systems sequestered carbon at 0.141-0.217 t-C/t-straw. The net energy ratio (NER) of the portable systems was higher than the centralized one at 10.29-16.26 compared to 6.04. For the centralized system, the carbon sequestration and the cumulative energy demand were most sensitive to the charcoal yield. Converting straw residues into charcoal can reduce GHG emissions by 80% after approximately 8.5 years relative to the baseline of in-field decomposition, showing these systems are effective carbon sequestration methods. (C) 2016 Elsevier Ltd. All rights reserved.