화학공학소재연구정보센터
Plasma Chemistry and Plasma Processing, Vol.36, No.5, 1211-1228, 2016
Carbon Dioxide Destruction with Methane Reforming by a Novel Plasma-Catalytic Converter
A novel plasma-catalyst converter (NPCC) was engineered in applying the carbon capture utilization technology for the destruction of carbon dioxide (CO2), which is a cause of global warming and is generated from the combustion of fossil fuels. The NPCC has an orifice-type baffle to improve an amount of gas feed with the higher CO2 destruction for a stationary point sources application . To examine its ability for the CO2 destruction, the performance analysis was conducted on the effects of methane additive, nozzle injection velocity, total gas feed, and catalyst type. The product gas from the NPCC was combustible components like CO, H-2, CH4, THCs. The CO2 destruction and the CH4 conversion at a 1.29 CH4/CO2 ratio were 37 and 47 %, respectively, and the energy decomposition efficiency was 0.0036 L/min W. The nickel oxide catalyst among other catalysts showed the most effectiveness for the CO2 destruction and CH4 conversion at a lower temperature. The carbon-black produced without the catalytic bed has carbon nanoparticles with diverse shapes, such as spherical carbon particles and carbon nanotubes; and its high conductivity and specific surface area were suitable for special electronic materials, fuel cells, and nanocomponents.