화학공학소재연구정보센터
Journal of Industrial and Engineering Chemistry, Vol.45, 248-256, January, 2017
Photocatalytic removal of cefazolin using Ag3PO4/BiOBr under visible light and optimization of parameters by response surface methodology
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The degradation of cefazolin (CFZ) by Ag3PO4/BiOBr composites under visible-light irradiation was explored. The main and interaction of parameters (catalyst dosage, pH, CFZ initial concentration and degradation time) on removal of CFZ were studied by Box-Behnken design combined with response surface methodology. The pH was the most influential factor and both h+ and ㆍOH played a role in the photocatalytic process. The high correlation coefficients (R2 = 0.9986 and adjusted R2 = 0.9973) demonstrated close fit between the predicted and experimental values. The exceptional efficiency of Ag3PO4/BiOBr composite in removing CFZ represents a promising technique for treatment of CFZcontaining wastewater.
  1. Zhang QQ, Ying GG, Pan CG, Liu YS, Zhao JL, Environ. Sci. Technol., 49, 6772 (2015)
  2. Fernandes R, Amador P, Prudencio C, Rev. Med. Microbiol., 24, 7 (2013)
  3. Bu QW, Wang B, Huang J, Deng SB, Yu G, J. Hazard. Mater., 262, 189 (2013)
  4. Leung HW, Minh TB, Murphy MB, Lam JC, So MK, Martin M, Lam PK, Richardson BJ, Environ. Int., 42, 1 (2012)
  5. Gulkowska A, Leung HW, So MK, Taniyasu S, Yamashita N, Yeung LWY, Richardson BJ, Lei AP, Giesy JP, Lam PKS, Water Res., 42, 395 (2008)
  6. Wang XH, Lin AY, Environ. Sci. Technol., 46, 12417 (2012)
  7. Gros M, Rodriguez-Mozaz S, Barcelo D, J. Chromatogr. A, 1292, 173 (2013)
  8. Zhang J, Meng J, Li Y, Hu C, Arch. Pharm. Chem. Life Sci., 343, 553 (2010)
  9. Jiang M, Wang L, Ji R, Chemosphere, 80, 1399 (2010)
  10. Guo R, Xie W, Chen J, Food Chem. Toxicol., 78, 116 (2015)
  11. Knapp CW, Dolfing J, Ehlert PAI, Graham DW, Environ. Sci. Technol., 44, 580 (2010)
  12. Nature 492, 2012, 314.
  13. Gilbert N, Nature, 81, 125 (2012)
  14. Fabbri D, Minella M, Maurino V, Minero C, Vione D, Chemosphere, 134, 452 (2015)
  15. Li LP, Wei DB, Wei GH, Du YG, J. Hazard. Mater., 262, 48 (2013)
  16. Lin AYC, Lin CF, Tsai YT, Lin HHH, Chen J, Wang XH, Yu TH, Water Sci. Technol., 62, 2450 (2010)
  17. Lin AY, Yu TH, Lin CF, Chemosphere, 74, 131 (2008)
  18. Rizzo L, Manaia C, Merlin C, Schwartz T, Dagot C, Ploy MC, Michael I, Fatta-Kassinos D, Sci. Total Environ., 447, 345 (2013)
  19. Fakhri A, Rashidi S, Asif M, Tyagi I, Agarwal S, Gupta VK, J. Mol. Liq., 215, 269 (2016)
  20. Li L, Wei D, Wei G, Du Y, Chemosphere, 149, 279 (2016)
  21. Gurkan YY, Turkten N, Hatipoglu A, Cinar Z, J. Chem. Eng., 184, 113 (2012)
  22. Pugazhenthiran N, Murugesan S, Anandan S, J. Hazard. Mater., 263, 541 (2013)
  23. Pugazhenthiran N, Murugesan S, Sathishkumar P, Anandan S, J. Chem. Eng., 241, 401 (2014)
  24. Mehraj O, Mir NA, Pirzada BM, Sabir S, Appl. Surf. Sci., 332, 419 (2015)
  25. Cui Z, Si M, Zheng Z, Mi L, Fa W, Jia H, Catal. Commun., 42, 121 (2013)
  26. Wang Y, Cheng X, Meng X, Feng H, Yang S, Sun C, J. Alloy. Compd., 632, 445 (2015)
  27. Cui ZK, Zhang FL, Zheng Z, Fa WJ, Huang BJ, Mater. Technol., 29, 214 (2014)
  28. Li YJ, Yu LM, Li N, Yan WF, Li XT, J. Colloid Interface Sci., 450, 246 (2015)
  29. Chong MN, Jin B, Chow CW, Saint C, Water Res., 44, 2997 (2010)
  30. Ahmed S, Rasul MG, Brown R, Hashib MA, J. Environ. Manage., 92, 311 (2011)
  31. Sakkas VA, Islam MA, Stalikas C, Albanis TA, J. Hazard. Mater., 175(1-3), 33 (2010)
  32. Ai CL, Zhou DD, Wang Q, Shao XW, Lei YJ, Sol. Energy, 113, 34 (2015)
  33. Mokhtar WNAW, Bakar WAWA, Ali R, Kadir AAA, J. Ind. Eng. Chem., 30, 274 (2015)
  34. Jia M, Hu X, Wang S, Huang Y, Song L, J. Environ. Sci., 35, 172 (2015)
  35. Yi ZG, Ye JH, Kikugawa N, Kako T, Ouyang SX, Stuart-Williams H, Yang H, Cao JY, Luo WJ, Li ZS, Liu Y, Withers RL, Nat. Mater., 9(7), 559 (2010)
  36. Zhao J, Chen C, Ma W, Top. Catal., 35, 269 (2005)
  37. Rauf MA, Meetani MA, Hisaindee S, Desalination, 276(1-3), 13 (2011)
  38. Wang K, Xu J, Hua X, Li N, Chen MD, Teng F, Zhu YF, Yao WQ, J. Mol. Catal. A-Chem., 393, 302 (2014)
  39. Li RP, Song XH, Huang YP, Fang YF, Jia MK, Ma WH, J. Mol. Catal. A-Chem., 421, 57 (2016)
  40. Gaya UI, Abdullah AH, J. Photochem. Photobiol. C, 9, 1 (2008)
  41. Sen R, Swaminathan T, Appl. Microbiol. Biotechnol., 47(4), 358 (1997)