화학공학소재연구정보센터
Journal of Industrial and Engineering Chemistry, Vol.47, 221-227, March, 2017
Hydrogenation of methyl methacrylate under mild conditions using biosynthesis Ru catalyst
E-mail:
Hydrogenation of methyl methacrylate (MMA) was investigated over Ru-based catalyst supported on active carbons (AC), which was prepared by bio-reduction method, using C. Platycladi (CP) leaf extract as reductant. By varying reaction temperature, hydrogen pressure and reaction time, hydrogenation of MMA over the biosynthesis Ru-based catalyst was carried out, and resulted the optimum conditions, 30 °C (room temperature), 2.0 MPa, and 50 min. The as-prepared Ru/AC catalyst showed high catalytic activity towards the hydrogenation of MMA, affording 100% of MMA conversion even under mild conditions without solvent and methyl isobutyrate was the only product.
  1. George V, Britto IJ, Sebastian MS, Radiat. Phys. Chem., 66, 367 (2003)
  2. George B, Maiti SN, Varma IK, J. Elastomers Plast., 38, 319 (2006)
  3. Ahn SH, Choi SI, Jung MJ, Nayab S, Lee H, J. Mol. Struct., 1113, 24 (2016)
  4. Huang YQ, Ma Y, Cheng YW, Wang LJ, Li X, Appl. Catal. A: Gen., 495, 124 (2015)
  5. Kelsey DR, Scardino BM, Grebowicz JS, Chuah HH, Macromolecules, 33(16), 5810 (2000)
  6. Osimitz TG, Eldridge ML, Sloter E, Welsh W, Ai N, Sayler GS, Menn FM, Toole C, Food Chem. Toxicol., 75, 188 (2015)
  7. Wienhofer G, Westerhaus FA, Junge K, Ludwig R, Beller M, Chem.-Eur. J., 19, 7701 (2013)
  8. Liu ZF, Ensor LC, Steinmetz JL, US Patent 20120149946A1, 2012.
  9. McCusker-Orth JE, Steinmetz JL, Messina AD, Perri ST, Liu ZF, Heidt PC, Tennant BA, US Patent 20080132742A1, 2008.
  10. Aldea R, Alper H, J. Organomet. Chem., 551, 349 (1998)
  11. Kim Y, Kim MJ, Bull. Korean Chem. Soc., 31, 1368 (2010)
  12. Natour S, Abu-Reziq R, RSC Adv., 4, 48299 (2014)
  13. Melo CI, Bogel-Łukasik R, da Silva MG, Bogel-Łukasik E, Green Chem., 13, 2825 (2011)
  14. Huo W, Zhang C, Yuan H, Jia M, Ning C, Tang Y, Zhang Y, Luo J, Wang Z, Zhang W, J. Ind. Eng. Chem., 20(6), 4140 (2014)
  15. Upare PP, Lee JM, Hwang DW, Halligudi SB, Hwang YK, Chang JS, J. Ind. Eng. Chem., 17(2), 287 (2011)
  16. Yabe Y, Sawama Y, Monguchi Y, Sajiki H, Catal. Sci. Technol., 4, 260 (2014)
  17. Zhu LH, Jiang YY, Zheng JB, Zhang NW, Yu CL, Li YH, Pao CW, Chen JL, Jin CH, Lee JF, Zhong CJ, Chen BH, Small, 11, 4385 (2015)
  18. Dauthal P, Mukhopadhyay M, J. Ind. Eng. Chem., 22, 185 (2015)
  19. Boudjahem AG, Redjel A, Mokrane T, J. Ind. Eng. Chem., 18(1), 303 (2012)
  20. Bogel-Łukasik E, Bogel-Łukasik R, da Ponte MN, Monatsh. Chem., 140, 1361 (2009)
  21. Ma Y, Huang YQ, Cheng YW, Wang LJ, Li X, Appl. Catal. A: Gen., 484, 154 (2014)
  22. Huang YQ, Ma Y, Cheng YW, Wang LJ, Li X, Catal. Commun., 72, 20 (2015)
  23. Ma Y, Huang YQ, Cheng YW, Wang LJ, Li X, Catal. Commun., 57, 40 (2014)
  24. Du B, Su H, Wang S, J. Ind. Eng. Chem., 21, 997 (2015)
  25. Zhu LH, Zheng JB, Yu CL, Zhang NW, Shu Q, Zhou H, Li YH, Chen BH, RSC Adv., 6, 13110 (2016)
  26. Xiong K, Li JL, Liew K, Zhan XD, Appl. Catal. A: Gen., 389(1-2), 173 (2010)
  27. Ni XJ, Zhang BS, Li C, Pang M, Su DS, Williams CT, Liang CH, Catal. Commun., 24, 65 (2012)
  28. Wang F, Yuan Z, Liu B, Chen S, Zhang Z, J. Ind. Eng. Chem., 38, 181 (2016)
  29. Helmer JC, Appl. Spectrosc., 23, 671 (1969)
  30. Upare PP, Lee M, Lee SK, Yoon JW, Bae J, Hwang DW, Lee UH, Chang JS, Hwang YK, Catal. Today, 265, 174 (2016)
  31. Choi SM, Seo MH, Kim H, Kim WB, Synth. Met., 161, 2405 (2011)
  32. Yan ZP, Lin L, Liu SJ, Energy Fuels, 23(8), 3853 (2009)
  33. Li BD, Wang C, Yi GQ, Lin HQ, Yuan YZ, Catal. Today, 164(1), 74 (2011)
  34. Li L, Zhu ZH, Yan ZF, Lu GQ, Rintoul L, Appl. Catal. A: Gen., 320, 166 (2007)
  35. Aouad S, Saab E, Aad EA, Aboukais A, Catal. Today, 119(1-4), 273 (2007)
  36. Du B, Su H, Wang S, J. Ind. Eng. Chem., 21, 997 (2015)
  37. Ren H, Xu CH, Zhao HY, Wang YX, Liu J, Liu JY, J. Ind. Eng. Chem., 28, 261 (2015)
  38. Bogel-Lukasik E, Wind J, Bogel-Lukasik R, da Ponte MN, J. Supercrit. Fluids, 54(1), 46 (2010)
  39. Bogel-Lukasik E, J. Supercrit. Fluids, 99, 121 (2015)