It has been argued that risk and performance-based approaches to licensing would be appropriate for Small Modular Reactors (SMRs) because their risk profiles differ from large-scale reactors. This is based on several factors including their limited electrical capacity of 300 MW, the below grade reactor vessel, and passive safety features. One design feature that can significantly reduce accident severity is the larger lateral surface area-to-volume (A/V) ratio of SMRs. Following a nuclear accident, this larger A/V ratio can increase the removal of radioactive particles due to natural phenomena compared to large light water reactors (LWRs). To quantify the improvements in safety, this work estimates the airborne radioactivity within containment and environmental dose exposure in a post-accident scenario for an advanced Generation III+ LWR (AP1000), a representative Generation II LWR (Surry), and an SMR On average, the AP1000, Surry, and SMR produces 139, 153, and 104 curies/ft(3) (182, 200, and 136 terabecquerels/m(3)) 75 min after a Loss-of-coolant-accident (LOCA). Using Monte Carlo simulations, the SMR produces less radioactivity per volume in containment than the AP1000 and Surry 84% and 96% of the time, respectively. On average, the AP1000, Surry, and SMR produces 84, 106, and 7 thousand curies/MWth (3.1, 3.9, and 2.5 petabecquerels/MWth) 75 min after a LOCA. The larger A/V ratio of the SMR plays a substantial role in reducing the radioactivity. While it is expected that the SMR would have a lower levels of radioactivity compared to the AP1000 and Surry, the SMR produces less radioactivity after normalizing by thermal reactor power and containment volume. With respect to environmental dose exposure, the US Environmental Protection Agency 1-5 rem (0.01-0.05 sieverts) Protective Action Guide (PAG) limits for whole body exposure is not exceeded at the 10-mile (16.1-km) EPZ using the mean estimates for the AP1000 and Surry. The iPWR does not exceed the 1 rem (0.01 sieverts) lower PAG limit for whole body exposure at the 5-mile (8-km) EPZ using the mean value. These findings can be used in conjunction with the improved analytical methods, found in the SOARCA study, to provide accurate and realistic estimates for exposure. This will help create a pathway to develop a regulatory basis for technology-neutral, risk-based approach to EPZs for iPWRs. (C) 2018 Elsevier Ltd. All rights reserved.