Selective desorption of transparent adhesive thin films using asymmetric distribution of vaporizable shell cross-linked nanocapsules

Intae Son; Byungsun Lee; Chi Hyeong Cho; Gi Tae Moon; Jeongho Hwang; Euiyun Jang; Bonghyun You; Jun Hyup Lee

Journal of Industrial and Engineering Chemistry, Vol.77, 477-483, September, 2019

DOI10.1016/j.jiec.2019.05.014 Export Citation

Selective desorption of transparent adhesive thin films using asymmetric distribution of vaporizable shell cross-linked nanocapsules

Intae Son, Byungsun Lee, Chi Hyeong Cho, Gi Tae Moon, Jeongho Hwang¹, Euiyun Jang¹, Bonghyun You¹, and Jun Hyup Lee^†

Department of Chemical Engineering, Myongji University, Yongin, Gyeonggi-do 17058, Republic of Korea
¹Next Generation R&D 1Team, Samsung Display, Yongin, Gyeonggi-do 17113, Republic of Korea

E-mail:

A selective desorption strategy for transparent adhesive thin films, using an asymmetric distribution of vaporizable shell cross-linked nanocapsules, is presented. The shell-crosslinked nanocapsules consist of an outer shell of polyacrylonitrile (PAN)/polymethylmethacrylate (PMMA) copolymer, and the inner core of a thermally vaporable methylcyclohexane. The vaporizable nanocapsule with a high PAN ratio exhibited excellent desorption efficiency after heat treatment owing to the gas barrier property of PAN. Transparent adhesive films with an asymmetric nanocapsule distribution in the vertical direction successfully realized selective and clean desorption at a specific interface, while maintaining high optical transmittance.

Keywords:Asymmetric distribution;Film detachment;Nanocapsule;Transparent adhesive thin film;Vaporization

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[1] Lanone S, Boczkowski J, Burr. Mol. Med., 6, 651 (2006)

[2] Taylor-Pashow KML, Rocca JD, Huxford RC, Lin W, Chem. Commun., 46, 5832 (2010)

[3] Miller MA, Weissleder R, Adv. Drug Deliv. Rev., 113, 61 (2017)

[4] Lacerda L, Bianco A, Prato M, Kostarelos K, Adv. Drug Deliv. Rev., 58, 1460 (2006)

[5] Long NV, Yang Y, Thi CM, Minh NV, Cao Y, Nogami M, Nano Energy, 2, 636 (2013)

[6] Zhou C, Liu Z, Du X, Mitchell DRG, Mai YW, Yan Y, Ringer S, Nanoscale Res. Lett., 7, 165 (2012)

[7] Jariwala D, Sangwan VK, Lauhon LJ, Marks TJ, Hersam MC, Chem. Soc. Rev., 42, 2824 (2013)

[8] Kamyshny A, Magdassi S, Small, 10, 3515 (2014)

[9] Zhang J, Lima FHB, Shao MH, Sasaki K, Wang JX, Hanson J, Adzic RR, J. Phys. Chem. B, 109(48), 22701 (2005)

[10] Aslan K, Wu M, Lakowicz JR, Geddes CD, J. Am. Chem. Soc., 129(6), 1524 (2007)

[11] Chen B, Deng J, Tong L, Yang W, Macromolcules, 43, 9613 (2010)

[12] Huang XY, Jiang PK, Adv. Mater., 27(3), 546 (2015)

[13] Qiu XP, Wu C, Macromolecules, 30(25), 7921 (1997)

[14] Liang Y, Gong JL, Huang Y, Zheng Y, Jiang JH, Shen GL, Yu RQ, Talanta, 72, 443 (2007)

[15] Joo SH, Park JY, Tsung CK, Yamada Y, Yang PD, Somorjai GA, Nat. Mater., 8(2), 126 (2009)

[16] Gao Y, Wang S, Luo H, Dai L, Cao C, Liu Y, Chen Z, Kanehira M, Energy Environ. Sci., 5, 6104 (2012)

[17] Peng XG, Schlamp MC, Kadavanich AV, Alivisatos AP, J. Am. Chem. Soc., 119(30), 7019 (1997)

[18] Soppimath KS, Tan DCW, Yang YY, Adv. Mater., 17(3), 318 (2005)

[19] Zhu J, Tang A, Law LP, Feng M, Ho KM, Lee DKL, Harris FW, Li P, Bioconjugate Chem., 16, 139 (2005)

[20] Lewis JS, Weaver MS, IEEE J. Sel. Top. Quant., 10, 45 (2004)

[21] Katchman BA, Smith JT, Obahiagbon U, Kesiraju S, Lee YK, Brien B, Kaftanoglu K, Christen JB, Anderson KS, Sci. Rep., 6, 29057 (2016)

[22] Pausan N, Liu Y, Lu Y, Hutchinson AR, J. Adhes., 93(10), 791 (2017)

[23] Banea MD, Silva LFM, Carbas RJC, Campilho RDSG, Int. J. Adhes. Adhes., 54, 191 (2014)

[24] Lu Y, Brouughton J, Winfield P, Int. J. Adhes. Adhes., 66, 33 (2016)

[25] Banea MD, da Silva LFM, Carbas RJC, Campilho RDSG, J. Adhes., 91(10-11), 823 (2015)

[26] Ryu C, Namura Y, Tsuruoka T, Hama T, Kaji K, Shimizu N, Dent. Mater. J., 30, 642 (2011)

[27] Zhang GH, Bon SAF, Zhao CY, Sol. Energy, 86(5), 1149 (2012)

[28] Kawaguchi Y, Itamura Y, Onimura K, Oishi T, J. Appl, Polym. Sci., 96, 1306 (2005)

[29] Gupta N, Rai R, Sikder A, Nandi S, Tanwar A, Khatokar R, Pask SD, Mitra S, RSC Adv., 6, 37933 (2016)

[30] Matyjaszewski K, Jo SM, Paik HJ, Gaynor SG, Macromolecules, 30(20), 6398 (1997)

[31] Sun D, Miyatake N, Sue HJ, Nanotechnology, 18, 215606 (2007)