International Journal of Hydrogen Energy, Vol.44, No.30, 15973-15984, 2019
Turbulent flame topology and the wrinkled structure characteristics of high pressure syngas flames up to 1.0 MPa
The turbulent flame topology characteristics of the model syngas with two different hydrogen ratios were statistically investigated, namely CO/H-2 ratio at 65/35 and 80/20, at equivalence ratio of 0.7. The combustion pressure was kept at 0.5 MPa and 1.0 MPa, to simulate the engine-like condition. The model syngas was diluted with CO2 with a mole fraction of 0.3 which mimics the flue gas recycle in the turbulent combustion. CH4/air flame with equivalence ratio of 1.0 was also tested for comparison. The flame was anchored on a premixed type Bunsen burner, which can generate a controllable turbulent flow. Flame front, which is represented by the sharp increased interface of the OH radical distribution, was measured with OH-PLIF technique. Flame front parameters were obtained through image processing to interpret the flame topology characteristics. Results showed that the turbulent flames possess a wrinkled character with smaller scale concave/convex structure superimposed on a larger scale convex structure under high pressure. The wrinkled structure of syngas flame is much finer and more corrugated than hydrocarbon fuel flames. The main reason is that scale of wrinkled structure is smaller for syngas flame, resulting from the unstable physics. Hydrogen in syngas can increase the intensity of the finer structure. Moreover, the model syngas flames have larger flame surface density than CH4/air flame, and hydrogen ratio in syngas can increase flame surface density. This would be mainly attributed to the fact that the syngas flames have smaller flame intrinsic instability scale l(i) than CH4/air flame. S-T/S-L of the model syngas tested in this study is higher than CH4/air flames for both pressures, due to the high diffusivity and fast burning property of H-2. This is mainly due to smaller L-M and l(i). V-f of the two model syngas is much smaller than CH4/air flames, which suggests that syngas flame would lead to a larger possibility to occur combustion oscillation. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.