Study on the forming mechanism and corrosion resistance of doping graphene composite film on the 6061 Al alloy

Mingming Ma; Yijun Cao; Qi Wang; Wei Shang; Ning Peng; Yuqing Wen

Journal of Industrial and Engineering Chemistry, Vol.107, 483-492, March, 2022

DOI10.1016/j.jiec.2021.12.020 Export Citation

Study on the forming mechanism and corrosion resistance of doping graphene composite film on the 6061 Al alloy

Mingming Ma, Yijun Cao, Qi Wang, Wei Shang, Ning Peng, and Yuqing Wen^†

Guangxi Key Laboratory of Electrochemical and Magnetochemical Function Materials, Guilin University of Technology, Guilin 541004, China

E-mail:

Flexible barrier films preventing corrosion are important for many industries ranging from engineering to medical to electronic materials. It is necessary to improve the corrosion resistance of aluminum alloys. The aluminum alloy sample reacted with sodium hydroxide was immersed in a double -[3-(triethoxylated) silicon-propyl] tetrasulfide and graphene（BTESPT/rGO) and cured in an oven at 100 °C to prepare a BTESPT/rGO composite film and discuss its film forming mechanism. The results shown that the film was dense and hydrophobic, which helped to improve the barrier properties of the film to corrosive ions, and its corrosion resistance was significantly better than that of a single BTESPT film. The corrosion current density of the BTESPT/rGO composite film was three orders of magnitude lower than that of the aluminum alloy substrate. The 240 h salt spray experiment shown that the BTESPT/rGO composite film greatly improved the corrosion resistance of the aluminum alloy substrate.

Keywords:Aluminum alloy;Graphene;Self-assembled film;Corrosion resistance

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[4] Wu SC, Hu YN, Duan H, Yu C, Jiao HS, Int. J. Fatigue, 91, 1 (2016)

[5] Yonetani H, Weld. Int., 22, 701 (2008)

[6] Zhe Z, Tian N, Zhang L, Ling W, Corrosion Sci., 98, 438 (2015)

[7] Mondal J, Marques A, Aarik L, Kozlova J, Simoes A, Sammelselg V, Corrosion Sci., 105, 161 (2016)

[8] Wei S, Chen B, Shi X, Chen Y, Xiao X, J. Alloy. Compd, 474, 541 (2009)

[9] Ansari KR, Quraishi MA, Singh A, Corrosion Sci., 95, 62 (2015)

[10] Winkler DA, Breedon M, White P, Hughes AE, Sapper ED, Cole I, Corrosion Sci., 106, 229 (2016)

[11] Narozny M, Zakowski K, Darowicki K, Corrosion Sci., 98, 605 (2015)

[12] Reza N, Adib KS, Ghasem HM, Prog. Org. Coat., 124, 110 (2018)

[13] Renaud A, Poorteman M, Escobar J, Dumas L, Paint Y, Bonnaud L, Dubois P, Olivier MG, Prog. Org. Coat., 112, 278 (2017)

[14] Shi L, Xu Y, Kang L, Yao Z, Wu S, Curr. Appl. Phys., 10, 719 (2010)

[15] Zhan X, Shang W, Wen Y, Li Y, Ma M, J. Alloy. Compd., 774, 522 (2019)

[16] Ding ZY, Cui LY, Chen XB, Zeng RC, Guan SK, Li SQ, Zhang F, Zou YH, Liu QY, J. Alloy. Compd., 764, 250 (2018)

[17] Wang D, Ni Y, Huo Q, Tallman DE, Thin Solid Films, 471, 177 (2005)

[18] Sheffer M, Groysman A, Mandler D, Corrosion Sci., 45, 2893 (2003)

[19] Wen Y, Meng HM, Wei S, RSC Adv., 5, 80129 (2015)

[20] Ramezanzadeh B, Bahlakeh G, Moghadam MHM, Miraftab R, Chem. Eng. J., 335, 737 (2017)

[21] Li Y, Gao W, Ci L, Wang C, Ajayan PM, Carbon, 48, 1124 (2010)

[22] Seger B, Kamat PV, J. Phys. Chem. C, 113, 7990 (2009)

[23] Tao Y, Chen M, Kong Q, Wang X, Guo X, Li W, Jiao K, Electrochim. Acta, 182, 1037 (2015)

[24] Yan Z, Wang L, Lu D, Shi X, Wang C, Duan X, Electrochim. Acta, 80, 77 (2012)

[25] Zhang, DongDong, Zhao, DongLin, Zhang, JiMing, Bai, LiZhong, J. Alloy. Compd., 589, 378 (2014)

[26] Zheng J, Lv H, Lin X, Ji G, Li X, Du Y, J. Alloy. Compd., 589, 174 (2014)

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[30] Sheng X, Cai W, Li Z, Xie D, Zhang X, Ind. Eng. Chem. Res., 55, 8576 (2016)

[31] Wen Y, Kong D, Shang W, Ma M, Zhan X, Colloids Surf. A: Physicochem. Eng. Asp., 562, 247 (2019)

[32] Ying H, Sarkar DK, Chen XG, Appl. Surf. Sci., 356, 1012 (2015)

[33] Wang MH, Li Q, Li X, Liu Y, Fan LZ, Appl. Surf. Sci., 448, 351 (2018)

[34] Liu J, Lei H, Li S, Mei Y, Appl. Surf. Sci., 327, 241 (2015)

[35] Zhu H, Yue L, Chen Z, Zhang Y, Liu X, Yin Y, Chen S, Surf. Coat. Technol., 304, 76 (2016)

[36] Wen YQ, Int. J. Electrochem. Sci., 14, 6018 (2019)

[37] Dalmoro V, dos Santos JHZ, Armelin E, Aleman C, Azambuja DS, Corrosion Sci., 60, 173 (2012)

[38] Yim H, Kent MS, Tallant DR, Garcia MJ, Majewski J, Langmuir, 21, 4382 (2005)

[39] Chen S, Cai Y, Zhuang C, Yu M, Song X, Zhang Y, Appl. Surf. Sci., 331, 315 (2015)

[40] Zhang Y, Zhu H, Zhuang C, Chen S, Wang L, Dong L, Yin Y, Mater. Chem. Phys., 179, 80 (2016)

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[42] Dun Y, Zuo Y, Appl. Surf. Sci., 416, 492 (2017)

[43] Li CQ, Zhu MY, Ou JF, Lu YL, Wang FJ, Li W, RSC Adv., 8, 29201 (2018)