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Catalysis Reviews-Science and Engineering, Vol.44, No.3, 455-498, 2002
Recent advances and future aspects in the low-temperature conversion of saturated hydrocarbons
A brief review on the advances and future aspects in the low-temperature activation of carbon-hydrogen and carbon-carbon bonds in hydrocarbons is presented. Particular attention is given to a catalyst formulation for low-temperature conversion of hydrocarbons. An efficient catalyst design method for low-temperature activation of saturated hydrocarbons has been worked out using metal evaporation techniques. The characteristic property of such catalysts is the presence of metal particles on the surface in an atomically dispersed state. Some of the prepared catalysts cause complete hydrocracking of alkanes and cycloalkanes at 423-463K.
Keywords:saturated hydrocarbons;low-temperature activation of C-H and C-C bonds;metal-complexes;supported metal-complexes derived from metal vapor;hydrocracking;isomerization;coupling of methane