화학공학소재연구정보센터
Journal of Physical Chemistry A, Vol.108, No.41, 8954-8960, 2004
Approaches to wave packet imaging using femtosecond ionization spectroscopy
Different methods to obtain information about the probability densities of vibrational wave packets in diatomic molecule are compared. More explicitly, we consider pump-probe ionization processes. Time-resolved photoelectron spectra and total ion yields as well as fragment ion distributions are calculated, and these different quantities are employed to reconstruct radial densities. It is shown that pump-probe ionization experiments are well suited for the mapping of vibrational wave packets.