Journal of Physical Chemistry B, Vol.109, No.29, 13854-13856, 2005
Optical control of coherent lattice motions probed by femtosecond electron diffraction
We report the study of laser-induced coherent lattice motions using femtosecond electron diffraction. The oscillations of Bragg peak positions associated with a damped lattice vibration along the surface normal were directly observed in real time and with sub-milli-angstrom spatial resolution. In addition, by using a pair of optical excitation pulses and varying their time delay and relative pulse intensities, we demonstrated the successful control of coherent lattice motions.