The absorption and desorption of carbon dioxide in aqueous monoethanolamine (MEA) was measured in a rotating packed bed of size 398 mm outside diameter, 156 mm inside diameter, and axial depth 25 mm. The effect of lean amine temperature (20 and 40 degrees C), peripheral rotor gravity (31 and 87 g), and various MEA concentrations were investigated. Using MEA concentrations above 30 wt % achieved lower CO2 penetration levels. This is particularly pronounced for the 100% MEA solution. Comparison with conventional columns showed the advantages of using rotating packed beds in terms of saving size and space and efficient operation.