Journal of Hazardous Materials, Vol.147, No.1-2, 618-624, 2007
Filtration of nano-particles by a gas-solid fluidized bed
The filtration of 80 nm SiO2 and Al2O3 particles in a gas stream using fluidized beds was studied. Silica sand and activated carbon (A.C.) were adopted as bed materials to filtrate 80 nm SiO2 and Al2O3 particles. The collected particles were elutriated from the fluidized bed, so the filtration was a dynamic process and the variations of the removal efficiency with time were studied. Experimental results showed that the filtrations of 80 nm SiO2 and Al2O3 particles with a bed material of silica sand were not dynamic processes but the filtration by A.C. was. The removal efficiencies for SiO2 and Al2O3 particles using silica sand as bed material were held steady and found to be equal, between 86 and 93%. A.C. is considered to be more efficient than silica sand because it has a high specific surface area. However, the experimental data yield conflicting results. The removal efficiency of Al2O3 particles fell from 92% initially to 80% at the end of test-a little lower than that obtained by filtration using silica sand. A higher voidage of A.C. than silica sand weakens the removal of nanoparticles since the diffusion mechanism dominates. The removal efficiency Of SiO2 by A.C. decayed from 83 to 40% with time passed. The huge differences between the filtration efficiency Of SiO2 and that of Al2O3 particles by A.C. was associated with the extensive segregation Of SiO2 and A.C. particles, which caused more SiO2 particles to move to the top of the bed, where they were elutriated. The weak inter-particle force for SiO2 decreased the removal efficiency also. (C) 2007 Elsevier B.V. All rights reserved.