Industrial & Engineering Chemistry Research, Vol.46, No.23, 7426-7435, 2007
Heat-transfer studies in packed-bed catalytic reactors of low tube/particle diameter ratio
This work describes a heat-transfer study conducted in two beds of low tube/particle diameter ratio (d(t)/d(p) approximate to 3) with almost the same diameter but different lengths, packed with catalyst spheres, operating in quasiadiabatic and nonadiabatic modes. The operation in the short bed in a quasi-adiabatic mode provided independent sets of experiments to estimate the effective thermal conductivity at various Reynolds numbers. This information was transferred successfully to model the short and long beds operating in a nonadiabatic mode. The modeling compares the classical approach to model heat transfer in a packed bed with no hydrodynamics, against those which include the hydrodynamics and a radial voidage profile, as well as the boundary layer approximation of this model. Modeling results showed that very similar predictions of radial and axial temperature profiles are obtained in all cases, making it difficult to discriminate between both model approaches.