화학공학소재연구정보센터
Journal of Power Sources, Vol.189, No.2, 1023-1031, 2009
Gas-liquid two-phase flow distributions in parallel channels for fuel cells
In the present study, gas-liquid two-phase flow in a parallel square minichannel system oriented horizontally and at an incline is studied under operating conditions relevant to fuel cell operations. Flow mal-distribution in parallel channels occurs at low gas and liquid flow rates. In general, high superficial gas velocities are required to ensure even flow distribution, and the minimum gas flow rates required to achieve even distribution depend on the liquid flow rates, channel orientation and experimental procedures. As the inclination angle is increased, a higher gas flow rate is required to ensure even gas-liquid flow distribution while flow channels inclined downward seems to help in improving the even How distribution. The presence of flow hysteresis phenomena indicate that multiple flow distributions exist at the same given flow conditions when the gas flow rates are varied in ascencling and descending manners. Flow mal-distribution and flow hysteresis are directly linked with flow stability. More specifically, the actual gas and liquid distribution in parallel channels is determined by the stability of mathematical solutions of mass and momentum balance equations and also the flow history. For the first time, the present work investigates flow distributions in fuel cell flow fields by accounting for two-phase flow conditions. In addition, a novel approach is introduced to ensure flow distributions and their stability through contour construction of isobars where unstable flow region can be identified, which can be used in the design of parallel channel flow fields, especially for fuel cells. (C) 2009 Elsevier B.V. All rights reserved.