Electrochimica Acta, Vol.56, No.21, 7312-7318, 2011
Evaluation of the hydrodynamic behaviour of turbulence promoters in parallel plate electrochemical reactors by means of the dispersion model
The hydrodynamic behaviour of electrochemical reactors with parallel plate electrodes is experimentally studied using the stimulus-response method either with an empty reactor or with different turbulence promoters. Theoretical results which are in accordance with the analytical and numerical resolution of the dispersion model for a closed system are compared with the classical relationships of the normalized outlet concentration for open systems and the validity range of the equations is discussed. The experimental results were well correlated with the dispersion model using glass beads or expanded plastic meshes as turbulence promoters, which have shown the most advantageous performance. The Peclet number was higher than 63. The dispersion coefficient was found to increase linearly with flow velocity in these cases. (C) 2011 Elsevier Ltd. All rights reserved.
Keywords:Dispersion model;Electrochemical reactors;Hydrodynamic behaviour;Parallel plate electrodes;Turbulence promoters