A series of polyurethane (PU)/talc composites modified by a high molecular weight hydroxyl-terminated polydimethylsiloxane (HTPDMS) were prepared. The effect of the talc content on the mechanical, wettability and tribological properties of the PU composites was studied. Tensile strength of the PU composites reached to the maximum after adding 5% talc. The water contact angles (CA) of the original surfaces and worn surfaces of the polyurethane composites were measured. The experimental results indicated that the contact angles of the worn surface increased after friction. The friction and wear experiments were tested on a MRH-3 model ring-on-block test rig at different sliding speeds and loads under dry sliding and water lubrication. Experimental results revealed that the talc contributed to largely improve the tribological properties of the PU composites. The coefficient of friction (COF) of the composites increased with increasing talc. Scanning electron microscopic (SEM) investigations showed that the worn surfaces of the talc filled PU composites were smoother than pure polyurethane under given load and sliding speed. (C) 2011 Elsevier B. V. All rights reserved.