| 초록 |
Nature utilizes solar energy for the synthesis of various compounds, which remains as a target model for the development of artificial photosynthetic system. In biocatalysis systems, enzymes catalyze and build intricate products with high specificity in environmentally benign conditions. Therefore, we developed the photocatalyst-redox enzyme coupled bioreactor system that exemplified solar synthesis in a simple heterogeneous system. Generating NADH in non-enzymatic light-driven process and coupling it to the enzymatic dark reaction catalysis for chemical synthesis via photobiocatalysis, the present work remains conceptually a novel model. Also it demonstrates successfully a new and potentially promising visible-light driven artificial photosynthesis system for the ultimate goal of utilization of solar energy in chemical synthesis. |
