Adsorbed benzene/toluene oxidation using plasma driven catalysis with gas circulation: Elimination of the byproducts

Xiaoqing Dang; Caihong Qin; Xuemin Huang; Jingjing Teng; Jiayu Huang

Journal of Industrial and Engineering Chemistry, Vol.37, 366-371, May, 2016

DOI10.1016/j.jiec.2016.03.051 Export Citation

Adsorbed benzene/toluene oxidation using plasma driven catalysis with gas circulation: Elimination of the byproducts

Xiaoqing Dang^†, Caihong Qin, Xuemin Huang, Jingjing Teng, and Jiayu Huang¹

School of Environmental and Municipal Engineering,, Xi’an University of Architecture and Technology, No. 13 Yanta Road, Xi’an, Shaanxi 710055, PR China
¹Research Center of Air Pollution Control Technology, Chinese Research Academy of Environmental Sciences, Beijing, 100012, PR China

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Adsorbed benzene/toluene on Ag-MnOx/γ-Al2O3 and Ag-MnOx-CoOx/γ-Al2O3 catalysts can be oxidised by non-thermal plasma with gas circulation. The results showed that the gas circulation system effectively avoided the emissions of VOCs caused by plasma desorption. After the gas was circulated for 90 min, compared to γ-Al2O3, the introduction of Ag-MnOx/γ-Al2O3 improved the COx yield by 33%, with CO2 selectivity close to 100%, and reduced the amount of O3 by 51%, while Ag-MnOx-CoOx/γ-Al2O3 inhibited N2O formation by 38% in comparison with γ-Al2O3. Furthermore, the elimination mechanisms of N2O, O3, and the byproducts on the surface of catalysts were studied.

Keywords:Plasma driven catalysis;Adsorbed benzene/toluene;Gas circulation;N2O

[References]

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Kuroki T, Hirai K, Kawabata R, IEEE Trans. Ind. Appl., 46, 672 (2010)
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Prieto P, Nistor V, Nouneh K, Oyama M, Abd-Lefdil M, Diaz R, Appl. Surf. Sci., 258(22), 8807 (2012)
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Assadi AA, Bouzaza A, Merabet S, Wolbert D, Chem. Eng. J., 258, 119 (2014)
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[Referenced By]

[1] Vandenbroucke AM, Morent R, De Geyter N, Leys C, J. Hazard. Mater., 195, 30 (2011)

[2] Everaert K, Baeyens J, J. Hazard. Mater., 109(1-3), 113 (2004)

[3] Thevenet F, Sivachandiran L, Guaitella O, Barakat C, Rousseau A, J. Phys. D-Appl. Phys., 47, 224011 (2014)

[4] Mok YS, Kim DH, Curr. Appl. Phys., 11(5), S58 (2011)

[5] Kim HH, Ogata A, Futamura S, Appl. Catal. B: Environ., 79(4), 356 (2008)

[6] Kuroki T, Hirai K, Kawabata R, IEEE Trans. Ind. Appl., 46, 672 (2010)

[7] Zhao DZ, Li XS, Shi C, Fan HY, Zhu AM, Chem. Eng. Sci., 66(17), 3922 (2011)

[8] Saulich K, Mueller S, J. Phys. D-Appl. Phys., 46, 045201 (2013)

[9] Shi C, Chen B, Li X, Crocker M, Wang Y, Zhu A, Chem. Eng. J., 200-202, 729 (2012)

[10] Sivachandiran L, Thevenet F, Rousseau A, Chem. Eng. J., 270, 327 (2015)

[11] Wang WZ, Wang HL, Zhu TL, Fan X, J. Hazard. Mater., 292, 70 (2015)

[12] Dang X, Huang J, Cao L, Zhou Y, Catal. Commun., 40, 116 (2013)

[13] Dang X, Huang J, Zhou Y, Zhang Q, Fresenius Environ. Bull., 22, 3070 (2013)

[14] Kim KJ, Ahn HG, Appl. Catal. B: Environ., 91(1-2), 308 (2009)

[15] Chandler BD, Schabel AB, Pignolet LH, J. Catal., 193(2), 186 (2000)

[16] Hevia MAG, Perez-Ramirez J, Appl. Catal. B: Environ., 77(3-4), 248 (2008)

[17] Kiwi-Minsker L, Bulushev DA, Renken A, Catal. Today, 110(3-4), 191 (2005)

[18] Pauleta SR, Dell’Acqua S, Moura I, Coord. Chem. Rev., 257, 332 (2013)

[19] Karuppiah J, Reddy EL, Reddy PM, Ramaraju B, Karvembu R, Subrahmanyam C, J. Hazard. Mater., 237-238, 283 (2012)

[20] Raju BR, Reddy EL, Karuppiah J, J. Chem. Sci., 125, 673 (2013)

[21] Tang XJ, Feng FD, Ye LL, Zhang XM, Huang YF, Liu Z, Yan KP, Catal. Today, 211, 39 (2013)

[22] Karuppiah J, Karvembu R, Subrahmanyam C, Chem. Eng. J., 180, 39 (2012)

[23] Kim HH, Teramoto Y, Sano T, Negishi N, Ogata A, Appl. Catal. B: Environ., 166-167, 9 (2015)

[24] Prieto P, Nistor V, Nouneh K, Oyama M, Abd-Lefdil M, Diaz R, Appl. Surf. Sci., 258(22), 8807 (2012)

[25] Waterhouse GIN, Bowmaker GA, Metson JB, Appl. Surf. Sci., 183(3-4), 191 (2001)

[26] Kuroki T, Fujioka T, Kawabata R, IEEE Trans. Ind. Appl., 45, 10 (2009)

[27] Liang WJ, Ma L, Liu H, Li J, Chemosphere, 92, 1390 (2013)

[28] Assadi AA, Bouzaza A, Merabet S, Wolbert D, Chem. Eng. J., 258, 119 (2014)

[29] Huang HB, Ye DQ, Leung DYC, Feng FD, Guan XJ, J. Mol. Catal. A-Chem., 336(1-2), 87 (2011)

[30] Abedi K, Ghorbani-Shahna F, Jaleh B, Bahrami A, Yarahmadi R, Haddadi R, Gandomi M, J. Electrost., 73, 80 (2015)

[31] Maxime G, Amine AA, Abdelkrim B, Dominique W, Environ. Sci. Pollut. Res. Int., 21, 13127 (2014)

[32] Trinh QH, Mok YS, Catal. Today, 256, 170 (2015)

[33] Harling AM, Glover DJ, Whitehead JC, Zhang K, Appl. Catal. B: Environ., 90(1-2), 157 (2009)

[34] Zheng C, Zhu X, Gao X, Liu L, Chang Q, Luo Z, Cen K, J. Ind. Eng. Chem., 20(5), 2761 (2014)