Efficient removal of La(III) from water by surface metal sequestration methodology using 5-azo-phenolate-8-hydroxyquinoline as a task designed sequestering material

Mohamed E. Mahmoud; Asmaa K. Mohamed

Journal of Industrial and Engineering Chemistry, Vol.63, 220-229, July, 2018

DOI10.1016/j.jiec.2018.02.018 Export Citation

Efficient removal of La(III) from water by surface metal sequestration methodology using 5-azo-phenolate-8-hydroxyquinoline as a task designed sequestering material

Mohamed E. Mahmoud^†, and Asmaa K. Mohamed

Faculty of Sciences, Chemistry Department, Alexandria University, P.O. Box 426, Ibrahimia 21321, Alexandria, Egypt

E-mail:

The present work explores an efficient depositive removal process of La(III) by 5-azo-phenolate-8- hydroxyquinoline (5AP-8HQ) using surface metal sequestration methodology (SMSM). Structural characterization of La(III)-complex was confirmed by different techniques. The highest surface coverage value 1597.4 μg/cm2 was recognized using pH 6.0, 0.01 mol L-1 La(III) and 76 cm2 surface area. The depositive removal of La(III) followed the Freundlich isotherm model (R2 = 0.9972) and the values of thermodynamic parameters assured spontaneous and endothermic processes. Furthermore, among the four investigated kinetics models, pseudo-second-order model (K2 = 1.15 g/mg min) yielded the best fit to describe the removal experimental data of La(III).

Keywords:Surface metal sequestration methodology (SMSM);Removal;La(III);5-Azo-phenolate-8-hydroxyquinoline (5AP-8HQ);Factors optimization

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[2] Bunzil J, Piguet C, Chem. Soc. Rev., 34, 1048 (2005)

[3] Zhu Y, Zheng Y, Wang A, Int. J. Biol. Macromol., 72, 410 (2015)

[4] Massari S, Ruberti M, Resour. Policy, 38, 36 (2013)

[5] Sastri VS, Bunzli JC, Rao VR, Rayudu GVS, Perumareddi JR, Modern Aspects of Rare Earths and Their Complexes, Elsevier, Amsterdam, 2003.

[6] Haldoraia Y, Rengaraj A, Ryuc T, Shinc J, Huhb YS, Hana Y, Mater. Sci. Eng. B-Solid State Mater. Adv. Technol., 195, 20 (2015)

[7] Ciopec M, Davidescu CM, Negrea A, Grozav I, Lupa L, Negrea P, Popa A, Chem. Eng. Res. Des., 90(10), 1660 (2012)

[8] Kondo K, Matsuo T, Matsumoto M, Hydrometallurgy, 152, 204 (2015)

[9] Guptaa NK, Sengupta A, Hydrometallurgy, 171, 8 (2017)

[10] Awwad NS, Gad HM, Ahmad M, Aly HF, Colloids Surf. B: Biointerfaces, 81, 593 (2010)

[11] Chen Q, J. Rare Earths, 28, 125 (2010)

[12] Atrees MS, Metwally E, Demerdash M, Salem H, J. Radiat. Res. Appl. Sci., 9, 207 (2016)

[13] Galhoum AA, Mahfouz MG, Abdel-Rehem ST, Gomaa NA, Vincent T, Guiba E, Nanomaterials, 5, 154 (2015)

[14] Gabor A, Davidescu C, Negrea A, Ciopec M, Grozav I, Negrea P, Duteanu N, J. Environ. Manage., 204, 839 (2017)

[15] Wu D, Gao Y, Zheng X, Chen Y, Wang Q, ACS Sustain. Chem. Eng., 4, 6732 (2016)

[16] Memon R, Memon SQ, Bhanger MI, El-Turki A, Hallam KR, Allen GC, Colloids Surf. B: Biointerfaces, 70, 232 (2009)

[17] Oliveira RC, Garcia O, Adv. Mater. Res., 71, 605 (2009)

[18] Birungi ZS, Chirwa EMN, Bioresour. Technol., 160, 43 (2014)

[19] Zeng GM, Wan J, Huang DL, Hu L, Huang C, Cheng M, Xue WJ, Gong XM, Wang RZ, Jiang DN, J. Hazard. Mater., 339, 354 (2017)

[20] Hu L, Wan J, Zeng G, Chen A, Chen G, Huang Z, He K, Cheng M, Zhou C, Xiong W, Laiab C, Xuab P, Environ. Sci.: Nano, 4, 2018 (2017)

[21] Wan J, Zhang C, Zeng GM, Huang DL, Hu L, Huang C, Wu HP, Wang LL, J. Hazard. Mater., 320, 278 (2016)

[22] De-Bashan L, Bashan Y, Water Res., 38, 4222 (2004)

[23] Mulkerrins D, Dobsona ADW, Colleranb E, Environ. Int., 30, 249 (2004)

[24] Mahmoud ME, Haggag SMS, Chem. Eng. J., 166(3), 916 (2011)

[25] Barakat MA, Arab. J. Chem., 4, 361 (2011)

[26] Mahmoud ME, Amira MF, Seleim SM, Mohamed AK, J. Chem. Eng. Data, 62(2), 839 (2017)

[27] Mishra S, Coord. Chem. Rev., 252, 1996 (2008)

[28] Mahmoud ME, Amira MF, Selim SF, Mohamed AK, J. Mol. Liq., 237, 455 (2017)

[29] Shubin S, Yue Y, Yubing C, Ding C, Cheng W, Wang X, Environ. Sci. Technol., 49, 4255 (2015)

[30] Krishnakumar V, Ramasamy R, Spectroc. Acta Pt. A-Molec. Biomolec. Spectr., 61, 673 (2005)

[31] Al-Shannag M, Al-Qodah Z, Bani-Melhem K, Qtaishat MR, Alkasrawi M, Chem. Eng. J., 260, 749 (2015)

[32] Munagapati VS, Kim D, Ecotoxicol. Environ. Saf., 141, 226 (2017)

[33] Wong C, Barford JP, Chen G, Mckay G, J. Environ. Chem. Eng., 2, 698 (2014)

[34] Martins RJ, Vilar EVJP, Boaventura RAR, Braz. J. Chem. Eng., 31, 229 (2014)

[35] Roy A, Adhikari B, Majumder SB, Ind. Eng. Chem. Res., 52(19), 6502 (2013)

[36] Ozacar M, Sengil IA, Turkmenler H, Chem. Eng. J., 143(1-3), 32 (2008)

[37] Mahmoud ME, Yakout AA, Elserw MIA, Osman MM, Clean Soil Air Water, 44, 1 (2016)

[38] Abas SNA, Ismail MHS, Kamal ML, Izhar S, World Appl. Sci. J., 28, 1518 (2013)

[39] Dada AO, Olalekan AP, Olatunya AM, Dada O, J. Appl. Chem., 3, 38 (2012)

[40] Foo KY, Hameed BH, Chem. Eng. J., 156(1), 2 (2010)

[41] Varala S, Kumari A, Dharanija B, Kbhargava S, Parthasarathy R, Satyavathi B, J. Environ. Chem. Eng., 4, 405 (2016)

[42] Aly H, Kerim FA, Kandil A, J. Inorg. Nucl. Chem., 33, 4340 (1971)

[43] Ferrah N, Abderrahim O, Didi MA, IOSR J. Appl. Chem., 7, 45 (2014)