In recent years, supercapacitors have received considerable research attention for energy storage systems due to their high-power density, fast charge-discharge processes, and long cycle life. The superior performance of supercapacitors is considerably dependent on the electrode materials. Among electrode materials, graphene balls (GBs) and their composites have recently attracted strong interest. They are considered ideal for the fabrication of electrode materials because of their unique characteristics of large specific surface area and superior electric conductivity, which should make them very effective for use in supercapacitors. In particular, GBs and their microstructured composites have recently been proven promising candidates for supercapacitor electrodes. Their unique 3D morphology provides highly porous graphene structures for decoration with active materials. In this perspective, recent studies were highlighted and discussed that focus on GBs and their composites for the potential energy storage devices called supercapacitors, (i.e., electric double layer capacitors and pseudocapacitors). (C) 2019 The Society of Powder Technology Japan. Published by Elsevier B.V. and The Society of Powder Technology Japan. All rights reserved.