화학공학소재연구정보센터
Journal of Industrial and Engineering Chemistry, Vol.31, 244-250, November, 2015
Role of microporosity of carbon produced from rice husks on electrochemical performance of Pt-Ru catalyst for direct methanol fuel cells
E-mail:
Activated carbon was synthesized from rice husks via chemical activation using different ratios of AC:KOH (1:1, 1:2, 1:3, and 1:4). Pt-Ru was deposited on the activated rice husks (A-RHs) by a chemical reduction method. The A-RH (1:3) exhibited a large surface area (>2000 m2/g) and high total pore volume (1.47 cm3/g), providing optimal conditions for Pt-Ru dispersion and subsequent improvement of electrochemical performances. Consequently, it was found that the electrochemical behavior of A-RH catalyst was improved by larger active surface area and optimal pore structure, suggesting new potential for rice husks as a superior direct methanol fuel cell catalyst.
  1. Tsujiguchi T, Abdelkareem MA, Kudo T, Nakagawa N, Shimizu T, Matsuda M, J. Power Sources, 195(18), 5975 (2010)
  2. Nakagawa N, Tsujiguchi T, Sakurai S, Aoki R, J. Power Sources, 192, 325 (2012)
  3. Feng C, Takeuchi T, Abdelkareem MA, Tsujiguchi T, Nakagawa N, J. Power Sources, 242, 57 (2013)
  4. Kim IT, Choi M, Lee HK, Shim J, J. Ind. Eng. Chem., 19(3), 813 (2013)
  5. Kim MS, Fang B, Chaudhari NK, Song M, Bae TS, Yu JS, Electrochim. Acta, 55(15), 4543 (2010)
  6. Park KW, Lee YW, Oh JK, Kim DY, Han SB, Ko AR, Kim SJ, Kim HS, J. Ind. Eng. Chem., 17(4), 696 (2011)
  7. Park KW, Sung YE, J. Ind. Eng. Chem., 12(2), 165 (2006)
  8. Wasmus S, Kuver A, J. Electroanal. Chem., 461(1-2), 14 (1999)
  9. Li XW, Liu JY, Huang QH, Vogel W, Akins DL, Yang H, Electrochim. Acta, 56(1), 278 (2010)
  10. Park SJ, Kim TJ, Lee JR, J. Polym. Sci. B: Polym. Phys., 38(16), 2114 (2000)
  11. Guo JS, Sun GQ, Wang Q, Wang GX, Zhou ZH, Tang SH, Jiang LH, Zhou B, Xin Q, Carbon, 44, 152 (2006)
  12. Liang YM, Zhang HM, Yi BL, Zhang ZH, Tan ZC, Carbon, 43, 3144 (2005)
  13. Zhang X, Chan KY, Chem. Mater., 15, 451 (2003)
  14. Wang ZB, Yin GP, Shi PS, Battery Bimonthly, 35, 70 (2005)
  15. Wang ZB, Yin GP, Shi PF, J. Power Sources, 163(2), 688 (2007)
  16. Liu HS, Song CJ, Zhang L, Zhang JJ, Wang HJ, Wilkinson DP, J. Power Sources, 155(2), 95 (2006)
  17. Jung MJ, Jeong E, Kim Y, Lee YS, J. Ind. Eng. Chem., 19(4), 1315 (2013)
  18. Mohammadi SZ, Hamidian H, Moeinadini Z, J. Ind. Eng. Chem., 20(6), 4112 (2014)
  19. Meng LY, Park SJ, Carbon Lett., 15, 89 (2014)
  20. Antolini E, Appl. Catal., 88, 1 (2009)
  21. Calvillo L, Gangeri M, Perathner S, Centi G, Moliner R, Lazaro MJ, Int. J. Hydrog. Energy, 36, 9806 (2011)
  22. Ahmadi R, Amini MK, Int. J. Hydrog. Energy, 36(12), 7275 (2011)
  23. Tsai MC, Yeh TK, Tsai CH, Int. J. Hydrog. Energy, 36(14), 8261 (2011)
  24. Santasalo-Aarnio A, Borghei M, Anoshkin IV, Nasibulin AG, Kauppinen EI, Ruiz V, Kallio T, Int. J. Hydrog. Energy, 37(4), 3415 (2012)
  25. Yang C, Wang D, Hu X, Dai C, Zhang L, J. Alloy. Compd., 448, 109 (2008)
  26. Muniandy L, Adam F, Mohamed AR, Ng EP, Microporous Mesoporous Mater., 197, 316 (2014)
  27. Im JS, Park SJ, Lee YS, J. Colloid Interface Sci., 314(1), 32 (2007)
  28. Park SJ, Kim KD, Carbon, 39, 1741 (2001)
  29. Rafiee E, Shahebrahimi S, China J. Catal., 33, 1326 (2012)
  30. Alvarez J, Lopez G, Amutio M, Bilbao J, Olazar M, Bioresour. Technol., 170, 132 (2014)
  31. Chen HB, Wang HB, Xue ZP, Yang LF, Xiao Y, Zheng MT, Lei BF, Liu YL, Sun LX, Int. J. Hydrog. Energy, 37(24), 18888 (2012)
  32. Kim S, Lee JR, Park SJ, Korean J. Chem. Eng., 46, 118 (2008)
  33. Kim S, Park SJ, J. Solid State Chem., 11, 821 (2007)
  34. Kim S, Park SJ, J. Power Sources, 159(1), 42 (2006)
  35. Tokarz W, Lota G, Fackowiak E, Czerwinski A, Piela P, Electrochim. Acta, 98, 95 (2013)
  36. Lee SY, Kim BJ, Park SJ, Energy, 66, 72 (2014)
  37. Tang YB, Liu Q, Chen FY, Chem. Eng. J., 203, 10 (2012)
  38. Lee SY, Kim BJ, Park SJ, J. Solid State Chem., 19, 258 (2013)
  39. Park SJ, Jang YS, Shim JW, Ryu SK, J. Colloid Interface Sci., 260(2), 259 (2003)
  40. Lueking AD, Pan L, Narayanan DL, Clifford CEB, J. Phys. Chem. B, 109(26), 12710 (2005)
  41. Park SJ, Kim KD, J. Colloid Interface Sci., 212(1), 186 (1999)
  42. Bernardo EC, Egashira R, Kawasaki J, Carbon, 35, 1217 (1997)
  43. Ahmed MJ, Theydan SK, J. Anal. Appl. Pyrolysis, 99, 101 (2013)
  44. Park KW, Choi JH, Kwon BK, Lee SA, Sung YE, Ha HY, Hong SA, Kim H, Wieckowski A, J. Phys. Chem. B, 106(8), 1869 (2002)
  45. Radmilovic V, Gasteiger HA, Ross PN, J. Catal., 154(1), 98 (1995)
  46. Kunz HR, Gruver GA, J. Electrochem. Soc., 122, 1279 (1975)
  47. Tang S, Vongehr S, He G, Chen L, Meng XJ, J. Colloid Interface Sci., 125, 375 (2012)
  48. Chen CS, Pan FM, Appl. Catal. B: Environ., 91, 663 (2003)
  49. Wang ZB, Yin GP, Zhang J, Sun YC, Shi PF, Electrochim. Acta, 51, 5695 (2006)
  50. Salgado JRC, Paganin VA, Gonzalez ER, Montemor MF, Tacchini I, Anson A, Salvador MA, Ferreira P, Figueiredo FML, Ferreira MGS, Int. J. Hydrog. Energy, 38(2), 910 (2013)